Abstract
The introduction of chemically unique groups into proteins by means of non-natural amino acids has numerous applications in protein engineering and functional studies. One method to achieve this involves the utilization of a non-natural amino acid by the cell's native translational apparatus. Here we demonstrate that a methionine surrogate, azidohomoalanine, is activated by the methionyl-tRNA synthetase of Escherichia coli and replaces methionine in proteins expressed in methionine-depleted bacterial cultures. We further show that proteins containing azidohomoalanine can be selectively modified in the presence of other cellular proteins by means of Staudinger ligation with triarylphosphine reagents. Incorporation of azide-functionalized amino acids into proteins in vivo provides opportunities for protein modification under native conditions and selective labeling of proteins in the intracellular environment.
MeSH Terms
Animals
Azides/chemistry
Biochemistry/methods
Blotting, Western
Electrophoresis, Polyacrylamide Gel
Escherichia coli/enzymology
Kinetics
Mass Spectrometry
Methionine/chemistry
Methionine-tRNA Ligase/chemistry
Mice
Models, Chemical
Models, Molecular
Peptides/chemistry
Protein Biosynthesis
Protein Conformation
Recombinant Fusion Proteins/chemistry
Temperature
Tetrahydrofolate Dehydrogenase/chemistry
Chemicals
Azides
Peptides
Recombinant Fusion Proteins
Methionine
Tetrahydrofolate Dehydrogenase
Methionine-tRNA Ligase
Authors & Affiliations
4 authors, click to expand affiliations / ORCID
Kiick Kristi L
Department of Polymer Science and Engineering, University of Massachusetts, Amherst, MA 01003, USA.
Saxon Eliana
Tirrell David A
Bertozzi Carolyn R
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Expanding the Scope of Protein Biosynthesis by Altering the Methionyl-tRNA Synthetase Activity of a Bacterial Expression Host Scott Ross was helpful in conducting the 1D TOCSY NMR experiments and Pratip Bhattachary is thanked for assistance in other NMR experiments. We are grateful to Yves Mechulam for a sample of plasmid pBSM547W305F and to Hieronim Jakubowski of UMDNJ-New Jersey Medical School, Newark, New Jersey, for plasmid pGG3. K.L.K. thanks the U.S. Department of Defense for a National Defense Science and Engineering Graduate Fellowship. This work was supported by grants from the Polymers and Genetics Programs of the National Science Foundation and from the U.S. Army Research Office.
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