Abstract
Pseudomonas sp. strain DNT degrades 2,4-dinitrotoluene (DNT) by a dioxygenase attack at the 4,5 position with concomitant removal of the nitro group to yield 4-methyl-5-nitrocatechol (MNC). Here we describe the mechanism of removal of the nitro group from MNC and subsequent reactions leading to ring fission. Washed suspensions of DNT-grown cells oxidized MNC and 2,4,5-trihydroxytoluene (THT). Extracts prepared from DNT-induced cells catalyzed the disappearance of MNC in the presence of oxygen and NADPH. Partially purified MNC oxygenase oxidized MNC in a reaction requiring 1 mol of NADPH and 1 mol of oxygen per mol of substrate. The enzyme converted MNC to 2-hydroxy-5-methylquinone (HMQ), which was identified by gas chromatography-mass spectrometry. HMQ was also detected transiently in culture fluids of cells grown on DNT. A quinone reductase was partially purified and shown to convert HMQ to THT in a reaction requiring NADH. A partially purified THT oxygenase catalyzed ring fission of THT and accumulation of a compound tentatively identified as 3-hydroxy-5-(1-formylethylidene)-2-furanone. Preliminary results indicate that this compound is an artifact of the isolation procedure and suggest that 2,4-dihydroxy-5-methyl-6-oxo-2,4-hexadienoic acid is the actual ring fission product.
MeSH Terms
Biodegradation, Environmental
Catechols/metabolism
Dinitrobenzenes/metabolism
Fatty Acids, Unsaturated/metabolism
Mass Spectrometry
Models, Biological
NAD(P)H Dehydrogenase (Quinone)/isolation & purification
NADP/metabolism
Oxidation-Reduction
Oxygen/metabolism
Pseudomonas/enzymology,metabolism
Quinones/metabolism
Toluene/analogs & derivatives,metabolism
Chemicals
2,4-dihydroxy-5-methyl-6-oxo-2,4-hexadienoic acid
4-methyl-5-nitrocatechol
Catechols
Dinitrobenzenes
Fatty Acids, Unsaturated
Quinones
2,4,5-trihydroxytoluene
Toluene
NADP
2-hydroxy-5-methylquinone
2,4-dinitrotoluene
NAD(P)H Dehydrogenase (Quinone)
Oxygen
Authors & Affiliations
3 authors, click to expand affiliations / ORCID
Haigler B E
Armstrong Laboratory, EQC-OL, Tyndall Air Force Base, Florida 32403-5323.
Nishino S F
Spain J C
References (16)
16 references, click to expand
-
Purification and characterization of a bacterial nitrophenol oxygenase which converts ortho-nitrophenol to catechol and nitrite.
J Bacteriol. 1988 Apr;170(4):1789-94
PMID: 3350791
-
Initial hydrogenation during catabolism of picric acid by Rhodococcus erythropolis HL 24-2.
Appl Environ Microbiol. 1992 Sep;58(9):2933-7
PMID: 1444408
-
Enzymatic oxidation of p-nitrophenol.
Biochem Biophys Res Commun. 1979 May 28;88(2):634-41
PMID: 37837
-
Degradation of 1,4-dichlorobenzene by a Pseudomonas sp.
Appl Environ Microbiol. 1987 May;53(5):1010-9
PMID: 3606087
-
Bacterial aromatic ring-cleavage enzymes are classified into two different gene families.
J Biol Chem. 1989 Sep 15;264(26):15328-33
PMID: 2670937
-
Construction of a Pseudomonas hybrid strain that mineralizes 2,4,6-trinitrotoluene.
J Bacteriol. 1993 Apr;175(8):2278-83
PMID: 8468288
-
Catabolism of 1,3-dinitrobenzene by Rhodococcus sp. QT-1.
Arch Microbiol. 1991;157(1):76-9
PMID: 1814279
-
Metabolism of resorcinylic compounds by bacteria: alternative pathways for resorcinol catabolism in Pseudomonas putida.
J Bacteriol. 1976 Mar;125(3):985-98
PMID: 942589
-
Pathway for Biodegradation of p-Nitrophenol in a Moraxella sp.
Appl Environ Microbiol. 1991 Mar;57(3):812-9
PMID: 16348446
-
Metabolism of arylsulphonates by micro-organisms.
Biochem J. 1968 Feb;106(4):859-77
PMID: 5637368
-
Biodegradation of 2,4-dinitrotoluene by a Pseudomonas sp.
Appl Environ Microbiol. 1991 Nov;57(11):3200-5
PMID: 1781682
-
The metabolism of cresols by species of Pseudomonas.
Biochem J. 1966 Nov;101(2):293-301
PMID: 5966268
-
Fluoride elimination from substrates in hydroxylation reactions catalyzed by p-hydroxybenzoate hydroxylase.
J Biol Chem. 1980 May 10;255(9):4189-97
PMID: 6768750
-
Diverse substrate range of a Flavobacterium pentachlorophenol hydroxylase and reaction stoichiometries.
J Bacteriol. 1992 May;174(9):2898-902
PMID: 1569020
-
Metabolism of resorcinylic compounds by bacteria: orcinol pathway in Pseudomonas putida.
J Bacteriol. 1976 Mar;125(3):975-84
PMID: 1254564
-
Cloning and characterization of Pseudomonas sp. strain DNT genes for 2,4-dinitrotoluene degradation.
J Bacteriol. 1993 Mar;175(6):1831-7
PMID: 8449889