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PMID: 2158301 Published · ppublish English Journal Article Research Support, Non-U.S. Gov't

Beta-lactamases as fully efficient enzymes. Determination of all the rate constants in the acyl-enzyme mechanism.

The Biochemical journal ·Vol. 266 ·No. 3 ·1990-03-15 ·Pages 853-61

Christensen H, Martin MT, Waley SG

Abstract

The rate constants for both acylation and deacylation of beta-lactamase PC1 from Staphylococcus aureus and the RTEM beta-lactamase from Escherichia coli were determined by the acid-quench method [Martin & Waley (1988) Biochem. J. 254, 923-925] with several good substrates, and, for a wider range of substrates, of beta-lactamase I from Bacillus cereus. The values of the acylation and deacylation rate constants for benzylpenicillin were approximately the same (i.e. differing by no more than 2-fold) for each enzyme. The variation of kcat./Km for benzylpenicillin with the viscosity of the medium was used to obtain values for all four rate constants in the acyl-enzyme mechanism for all three enzymes. The reaction is partly diffusion-controlled, and the rate constant for the dissociation of the enzyme-substrate complex has approximately the same value as the rate constants for acylation and deacylation. Thus all three first-order rate constants have comparable values. Here there is no single rate-determining step for beta-lactamase action. This is taken to be a sign of a fully efficient enzyme.

MeSH Terms
Acylation Bacillus cereus/enzymology Cephalosporins/metabolism Chemical Phenomena Chemistry Deuterium Escherichia coli/enzymology Hydrolysis Kinetics Penicillanic Acid/pharmacology Penicillin G/metabolism Staphylococcus aureus/enzymology Substrate Specificity beta-Lactamase Inhibitors beta-Lactamases/metabolism
Chemicals
Cephalosporins beta-Lactamase Inhibitors Penicillanic Acid Deuterium 6-iodopenicillanic acid beta-Lactamases nitrocefin Penicillin G
Authors & Affiliations
3 authors, click to expand affiliations / ORCID
Christensen H
Sir William Dunn School of Pathology, University of Oxford, U.K.
Martin M T
Waley S G
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34 references, click to expand
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Article Info
Journal
The Biochemical journal
Abbr.
Biochem J
ISSN
0264-6021
Published
1990-03-15
Pages
853-61
Language
English
Region
England
NLM ID
2984726R
PMCID
PMC1131217
Subset
IM
Corrections
ErratumIn
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CommentIn
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